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Atmospheric Environment
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Special Issue:Sixth Scientific Conference of the International Global Atmospheric Chemistry Project (IGAC) Bologna, Italy; 13–17 September 1999
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The study concerning carbon dioxide measurements taken during the 1997, 1998 and 1999 summer campaigns at two different altitude stations and biospheric conditions are presented. The higher station (Mt. Cimone, 2165 m a.s.l.) is characterised by 360° free horizon and is located on a rocky mountain while the lower (Ninfa lake, 1550 m a.s.l.) is located inside the red spruce and beech forest. The different behaviour of CO2 at the two mountain stations has been registered. It shows the strong effect of nighttime soil emission and vegetation respiration on CO2 mixing ratio increases and of diurnal vegetative activity on CO2 concentration decreases at the lower measurement site. The baseline character of the higher measurement site has been confirmed by comparison of CO2 diurnal amplitudes recorded at the two stations.
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In order to evaluate the background ozone concentration at Mt. Cimone (2165 m a.s.l.), the contribution of air masses characterised by different provenances is analysed in this paper. The analysis method is based on identification of background air masses which travelled above the 780 hPa pressure level for at least 48 h before arriving at Mt. Cimone. Not being recently mixed with boundary layer air, these air masses are characterised by a chemical age greater than 2 days. This analysis has shown that under background conditions the yearly principal maximum of ozone is recorded in spring and a secondary maximum is recorded in summer. In contrast, if we consider non-background conditions, the principal maximum is found in late summer and a secondary one in spring. In addition, the analysis indicates the presence of a smooth latitudinal gradient of background ozone concentrations in air masses arriving at Mt. Cimone, with higher concentrations coming from the north and lower ones from the south.
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Chlorofluorocarbons and their replacement compounds are anthropogenic compounds of great environmental concern. For this reason monitoring their atmospheric mixing ratios on a worldwide scale is recommended. An analytical methodology for the simultaneous determination of selected chlorofluorocarbons and their replacement compounds has recently been developed. This methodology was applied in the analysis of actual air samples collected in remote and semi-remote areas located in the Northern and Southern Hemispheres. The concentration levels measured in the air samples collected in the two hemispheres are reported.